Lavender Town Music.
I actually used to have the original Pokemon Green (in Japanese) on my GBA when I was kid, and remember playing through lavender town, and it used to creep me out so much, and it still does.
Imagine playing the original music at 4 am after you've just watched a horror movie, or something. x_x
What VG music creeps you out?
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The description doesn't fit, if not a synonym of menace